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Increasingly during modern times our educational aims are directed toward elevating knowledge at a cost of marginalizing mystery. The following philosophical paper argues for a doctrine of mystery, by exploring what mystery is, its relationship with knowledge, the history of its marginalization, and the implications this has for education writ large, with a focus on environmental education research and praxis. A comprehensive literature review of mystery from philosophical, scientific, and theological perspectives, and its synthesis and analysis has generated a topology of domains, realms, and senses of mystery underscoring the conclusion that a doctrine of mystery is important for ontological, epistemological, and ecological reasons.