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Psychological Capital (PsyCap) is a key element of positive psychology and has been identified as a “missing piece” in contemporary careers. PsyCap contains some specific characteristics that are critical to career development and has a positive influence on several work outcomes. One potential relationship that has not been well documented in the literature is between PsyCap and work values. We investigate this association among 2,052 Canadians, aged 14 to 36. Descriptive statistics, multiple linear regression, and logistic regression models confirm the strong relationship between participants’ PsyCap and intrinsic work values, specifically among females and younger employees. Understanding this relationship can provide managers with practical implications in three major areas in human resource management: employee recruitment, engagement, and retention.