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Based on expectancy-value and dimensional comparison theory, domain-specific motivational beliefs (e.g., self-concept) are important predictors of adolescents’ career aspirations. However, we know relatively little about how domain-specific career aspirations evolve across adolescence, and whether they predict future domain-specific motivation. This study used longitudinal data from Germany (N=8,289) to evaluate the stability, trajectories, and predictors for math- and reading-related career aspirations. Further, we investigated whether within- and cross-domain associations to self-concept and motivation change over time, as well as if career aspirations predict future self-concept and motivation. We observed increasing stability and importance levels of math- and reading-related career aspirations. We found longitudinal within- and cross-domain effects mainly for the reading domain, and discuss implications for career orientation.