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This study examined how instructional leadership practices by directors in early care and education (ECE) settings were associated with teacher outcomes, specifically teachers’ engagement in collaborative job-embedded professional learning (JEPL) and commitment to the workplace. We analyzed data from 22 center-based ECE programs (teacher N = 284) and found that effective instructional leadership was associated with improved relational coordination as perceived by teachers; relational coordination, characterized by shared goals and knowledge, mutual respect, and high-quality communication, mediated the relationship between leadership practices and positive teacher outcomes. These results highlight the importance of fostering relational coordination to enhance teacher engagement and commitment, offering critical insights for developing leadership programs that improve both teacher and program outcomes in ECE settings.