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This study investigated the interplay between social self-concept, social perspective-taking, and peer relationships in fourth- and fifth-graders in the context of an intervention designed to enhance students’ social perspective-taking through collaborative activities. Multiple group structural equation modeling revealed differences between the treatment and control groups. In the treatment group, higher levels of students’ social perspective-taking mediated the relationship between social self-concept and improved peer relationships, resulting in lower physical and relational aggression and higher friendship. In the control group, social perspective-taking only mediated the relationship between social self-concept and reduced physical aggression. These findings highlight the importance of social perspective-taking as a mechanism of collaborative learning in fostering positive peer relationships in educational settings.