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This study proposes a multimodal online learning experience measurement model based on Long Short-Term Memory (LSTM) networks to address the subjectivity and time delays of traditional self-report methods. By integrating eye-tracking, EEG, and facial expression data, a deep feature representation framework was constructed. High-precision instruments captured synchronized physiological–behavioral signals, with labeled questionnaire data used for supervision. A sliding window strategy enhanced temporal resolution and model generalizability. The LSTM model achieved 91.66% accuracy, outperforming conventional algorithms. This approach enables real-time monitoring and dynamic feedback, supporting personalized and adaptive learning strategies, and offers a scalable solution for intelligent assessment in online education.