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Transportation electrification is crucial for reducing pollution and climate change. While market incentives drive new energy vehicle adoption, the effectiveness of China's unique command-and-control regulations in the car-sharing market is less studied. We implement a quasi-natural experiment by using the city-level administrative mandates, which establish new energy vehicles as ride-hailing registration prerequisites. Employing a staggered DID approach and an instrumental variables approach, we quantify these policies' causal effects on rental vehicle sales. The results show that command-and-control regulation can significantly promote the electrification transition in the car sharing market, leading to a 64.4% increase in the sales of new energy rental cars. It has a more pronounced effect in western regions, non-central cities, and resource-based cities. The policy works by expanding charging infrastructure, increasing brand variety, and promoting urban-rural equality. Its impact is stronger in cities with high climate policy uncertainty, strong governmental environmental focus, and high innovation. Our results also show that this command-and-control regulation has a stronger boosting effect on pure electric rental cars and a dampening effect on other fuel-type new energy rental cars such as hybrids. It is worth noting that command-and-control regulations may generate negative externalities. While increasing the sales volume of new energy rental vehicles, they could simultaneously lower the overall quality of vehicles circulating in the market. Command-and-control regulations may also generate negative spatial spillover effects, reducing sales of new energy rental vehicles in surrounding cities. Our findings confirm the positive role and other multi-dimensional impact of command-and-control policy in car-sharing electrification and offer insights for transportation electrification policy design.