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Since the middle 1980s, desistance has become an increasingly studied topic among criminologists attempting to explicate processes that generate the abandonment of crime across the life-course. Despite considerable evidence that most offenders eventually mature out of delinquent behavior, several fundamental issues remain unresolved. One major issue involves the idea that criminality, often referred to as self-control in the criminological literature, can be a subject of changeability in producing the process underlying desistance from crime. In this paper, devoted to a recent application of the dual-process approach to decision-making brought about by the study of psychology and neuroscience, I attempted to answer this unsolved question by focusing on the important role of agency (choice) as a key to the explanation of the self-control development and associated changes in criminal behavior. Specifically, I provided how human agency can be conceptualized and explained in relation to the concept of self-control and investigated this concept into two forms of action control, goal-directed and habitual decision-making.