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This study examined the associations among social comparison, Facebook use, and psychological outcomes represented by mental health and perceived social support. In addition, the role of self-esteem and impression management was explored as antecedents of social comparison on Facebook. Using a sample of college students (N = 313) and structural equation modeling analyses, the study found a positive association between social comparison and Facebook use as well as a negative association between social comparison and mental health. However, there was no significant association between social comparison and perceived social support. In addition, Facebook use was positively associated with perceived social support, yet it was not significantly associated with mental health. Finally, both self-esteem and impression management were positively associated with social comparison on Facebook. Theoretical implications and limitations were discussed.