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With increasing calls for self-regulated learning (SRL), allowing students to become meta-cognitively and affectively engaged in learning, this study investigated the impact of three SRL programs: Holistic, combining Meta-Cognition + Meta-Affect (MA+MC), MC and MA alone, compared to a Control group on (a) Meta-cognition and Meta-affect, and (b) Solving mathematical problems with a novel task. Mixed-methods analysis with thinking-aloud protocols indicated that the SRL groups outperformed the control group. The Holistic group effectively used SRL processes by combining metacognitive and affective thinking paths, and demonstrated higher self-efficacy and problem solving. The MC group was more successful in the meta-cognitive aspect, and the MA group in reducing their negative emotions. No differences were found between the two groups in problem solving.