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Scholarship on community level structural disadvantage in the US context has long debated the role of segregation and racial composition in shaping neighborhood wellbeing. We consider extant theoretical perspectives on the association of Black population concentration in urban neighborhoods with both collective efficacy (mutual trust combined with the conjoint capacity to intervene on behalf of shared goals) and violent crime. We then test varying expectations on these associations drawing on data from the 2014-16 Columbus, Ohio-based Adolescent Health and Development in Context study in combination with American Community Survey data on neighborhood structural characteristics, and administrative data on violent crime rates. Contrary to prevailing assumptions regarding Black-concentrated urban neighborhoods, we find that, net of economic disadvantage, increasing proportion Black is associated with reduced collective efficacy and increased violent crime only at low baseline levels of Black population presence. Beyond a threshold, increasing neighborhood proportion Black is associated with increases in collective efficacy and declines in violent crime.