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Curiosity may be an overlooked concept in criminological theory. We previously found that curiosity predicted involvement in “exploratory” deviant/delinquent behavior, as theoretically expected (Mayone & Arneklev, 2015). These are behaviors that someone might engage in “a few times” (e.g., to satisfy their curiosity). Additional analyses revealed that curiosity also significantly predicted a general crime/deviance index (Arneklev & Dario, 2018A) and specific serious offenses (Arneklev & Dario, 2018B), while controlling for self-control capacity (Gottfredson & Hirschi, 1990). Here, we test curiosity’s ability to predict deviant/delinquent behavior by including “more than a few times” as an attribute in our dependent variable, again controlling for the most powerful and widely used self-control capacity scale, the Grasmick scale (Pratt & Cullen, 2000). Implications of significant results, and future directions, are discussed.